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The correspondence chiefly consists of forty-nine letters written by Jerome while a student at Mount Holyoke College, 1907-1911. Her correspondence is addressed to her mother, Elizabeth Maude Jerome, grandmother Elizabeth Gilbert Jerome, and brother Gilbert Nelson Jerome, and most of the letters date from 1907-1909. She describes many aspects of her life at Mount Holyoke, including traditions such as Mountain Day, Freshman Frolic, and Junior Show, and activities such as parties, concerts, basketball games, an "Ice Carnival," play performances, try-outs for the College Choir, and a mock political convention and parade of suffragists held in November 1908. She also discusses religious services, her clothing and finances, and Mount Holyoke's food and grading policies. Many letters mention friends, classmates, and faculty members and administrators, particularly President Mary Emma Woolley and botany professor Henrietta Edgecomb Hooker. In another letter to her mother dated April 17, 1914, Jerome comments on her brother's "new position" and describes a recent visit to Boston. The correspondence also includes postcards and letters, 1940-1979, from several Mount Holyoke College friends and classmates in which they discuss their activities. In addition, a letter from 1979 concerns her contribution to the "GOP Victory Fund of the Republican Congressional Committee."

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Most of the material in this scrapbook relates to Jerome's years as a student at Mount Holyoke College, 1907-1911. The volume contains notes from friends and faculty members and copies of many College publications, including programs for plays, concerts, and ceremonial events such as Founder's Day. A "Table of Measurements" in the scrapbook gives Jerome's physical dimensions and lung capacity in 1907 and 1910. The book also contains "Basket-Ball Songs," material relating to Senior Mountain Day in 1911, a laundry list, several of Jerome's report cards and examinations, newspaper clippings about events at the College, programs for plays, concerts, and church services in Amherst and Springfield, Massachusetts, and New Haven, Connecticut, dance cards, postcards, valentines and other greeting cards, and poems and drawings by Jerome. Photographs in the scrapbook are of friends and classmates, the campus, and faculty members, including botany professor Henitetta Edgecomb Hooker. Material dating from 1912-circa 1914 consists of her account of a friend's wedding, a postcard, programs, newspaper clippings, a pamphlet relating to Mount Holyoke College, and several photographs of classmates.

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Writings consists of stories, essays, and a poem written by Jerome. Most of the series consists of her short stories as published in issues of the New Haven High School monthly magazine "The Crescent" for 1904-1907. This series also includes a poem entitled "Autumn," dated September 1, 1912, an account of a visit to the "ancient home of the Gilberts" in England in 1924, and an essay called "Years Ago," written for the "New Haven Teachers' Journal" of December 1947 in which she recalls her years as a high school student.

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The artwork consists of two undated drawings by Jerome that were probably done between 1907 and 1939. One is a watercolor drawing of a child standing under a tree. The other is a silhouette of her mother, Elizabeth Maude Jerome.

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The memorabilia consist of the songbook for the Class of 1911 Junior Show at Mount Holyoke College, 1910; a catalogue for an exhibition of works by Jerome and other members of the New Haven Paint and Clay Club, Inc., in March 1936; an invitation to a tea honoring Jerome on the occasion of her retirement from the New Haven Library in 1952; and a note from "Tony" that accompanied his gift of a book of poems by John Updike, 1958.

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The oral history transcript consists of a typed transcript of interviews of Jerome conducted by Roberta Yerkes Blanshard in January and March 1975 for the New Haven Quota Club. Jerome discusses her ancestry tracing the Jerome and Gilbert family lines to the eighteenth century, and mentions her father, Yuan Phou Lee. She also describes her years as a student at Mount Holyoke College and her work in the New Haven library system.

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The biographical information chiefly consists of newspaper clippings about Jerome dating from 1922 and 1952-1963. These articles concern her work as Art and Music Librarian at the New Haven Main Branch Library from 1922-1952, her interest in the Boy Scouts of America, and her involvement with activities and events relating to Mount Holyoke College. Two articles from 1941 and 1944 review art exhibits in New Haven that included portraits by her. This series also includes a biographical note from about 1918, an obituary for Jerome, 1979, and tributes written after her death.

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The mah jong game that belonged to Jerome probably dates from the 1920s and includes tiles, dice, game pieces, and score sheets. The game, which is in its original container, was manufactured in the United States by the Milton Bradley Company. An instruction booklet with the game was written by J.P. Babcock and published by Parker Brothers, Inc. in 1923.

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The photographs chiefly consist of formal and informal images of Jerome from 1907-1952. Included are formal photographs of Jerome in her cap and gown when she graduated from Mount Holyoke College in 1911 and prints of photographs used in a newspaper article about her retirement from the New Haven Library in 1952. Informal photographs consist of one of Jerome as a young woman, possibly taken before she entered Mount Holyoke in 1907, and several taken later in life. This series also includes a 1945 photograph of "Catherine, Ethel Jackson, and Davis Jackson."